Meteo 532 -- Atmospheric
Chemistry -- Fall 2002
Final Take-home
Examination
assigned: 02
December 2002
due: 16 December 2002
Please keep your answers brief. As Strunk and White say: “Omit needless words.” If you think
that you need additional values for parameters to solve the problems,
assume reasonable values and state your assumptions. Please use JPL for any rate coefficients
that you might need. You can use any
books or notes, but please work alone.
1. (10 points)
Catalytic stratospheric ozone production. Consider the catalytic cycle:
ClO + O ®
Cl + O2
Cl
+ O3 ® ClO +
O2
net: O + O3 ®
2O2
.
In the
expression or ozone loss, we can write: d[O3] / dt = -2 kClO+O
[ClO][O].
Why can’t we
write this expression as: d[O3]
/ dt = - 2 kCl+O3 [Cl] [O3]?
2. (25 points)
Tropospheric ozone production.
a) Write down the expression for the net tropospheric ozone
production:
d[O3]/dt = P-L=?
b) We know that ozone
is actually produced from NO2+hv -->NO+O, followed by O+O2+M -->O 3+M. Why does the expression for d[O3]/dt
contain no terms for these two reactions?
c) What is the net ozone production rate, in
ppb hr-1, at 10 km altitude if NO=200 pptv, HO2 =5 pptv,
OH=0.5 pptv, O3=60 ppbv, H2O=200 ppmv,
and JO3=2x10-5 s-1? Assume also the p=250 mb and T=235 K and that [RO2]
is negligible.
d) Consider the set
of reactions:
OH+CO -->H+CO 2
H+O2+M--> HO2+M
OH+O3 -->HO2+O2
HO2+NO -->OH+NO2
HO2+O3 -->OH+2O2
Write down the rate equation for OH,
assuming that the second reaction is much faster than the others.
e) Assuming that OH
and HO2 are in steady-state, write down the [HO2]/[OH]
ratio in terms of [NO], [CO], [O3], and the rate coefficients.
3. (10 points) The aircraft industry recently considered
creating a fleet of 500-1000 High-Speed Supersonic Civilian Transports (HSCTs)
that would carry passengers across the oceans in about ˝ of the time of
existing subsonic aircraft. It was
estimated that these aircraft would double the NOx in the lower
stratosphere. An environment study
indicated that, if these aircraft flew below 18 km, ozone destruction would be
minimal. Use the attached schematic to
explain why so much pollutant might have so little effect on ozone.
4. (15 points) Aerosol size distributions. Explain why, in a collection of aerosols,
the larger ones generally have more mass than the smaller ones, even though the
smaller ones are more numerous. How
should a aerosol number distribution vary as a function of size in order for
the mass to be independent of size?
5. (25 points) An urban pollution plume comes into
equilibrium with clouds that have a liquid water content of 1 g m-3. The initial equilibrium values for SO2
is 20 ppbv and for HNO3 is 0.01 pptv. The atmospheric pressure is 1013 hPa and the temperature is 298
K. Assume no CO2. We assume that all the HNO3 in
the aqueous phase is in the form of nitrate (NO3-), and
that HHNO3 = 2.1x105 M/atm and that the equilibrium
constant between HNO3·H2O Ű NO3-
+ H+ is 15.4 M.
a) What is the equation for the ion balance?
b) What is the initial pH of the clouds?
c) What fraction of the acidity is due to S(IV)
and what fraction is due to NO3-?
Assume that all the S(IV) in both the aqueous
and gas phase is reacted to S(VI) and all the NOx is reacted to HNO3. Assume that all the S(VI) is in the aqueous
phase. Note that the amount of NO3-
depends on [H+].
d) What is the new pH of the clouds?
e) What fraction of the acidity is due to S(VI)
and which fraction is due to NO3-?
Is [NO3-] now
different from its initial value?
6. (15 points) Ozone
isopleth diagram.
(a) Ozone isopleths are usually
plotted with VOCs on the x-axis and NOx on the y-axis. Yet we know that ozone production really
comes from the reaction of NO with HO2
and RO2. How are VOCs and NOx
related to ozone production? (Or put another way, what other information do
we need to know to get quantitative numbers of ozone production from VOC oxidation?)
(b) Briefly explain why the EPA has
been regulating only VOC emissions in an effort to reduce O3 in
urban areas.
(Super Bonus - 30 pts
) Variation of ozone production with
[NO]. HOx, the sum of OH+HO2,
has the rate equation:
d[HOx]/dt = P(HOx)
– {2kHO2+HO2[HO2 ][HO2] + 2kOH+HO2[OH][HO2]
+ kOH+NO2+M [M][NO2][OH]}
where P(HOx) is the production rate (molecules cm-3
s-1) of HOx, OH or HO2 and the three
expressions in brackets are three loss mechanisms for HOx. HO2+HO2 -->HOOH+O 2 dominates when NO
is low, OH+HO2 -->H2O+O2 dominates when NO
is about 100 pptv, and OH+NO2+M --> HNO3+M dominates when NO
is greater than a few hundred ppt. In
each one of these three NO regimes, we can assume that only the dominant HOx
loss reaction is occurring.
Using the equations in 2.d) to help
relate OH to HO2 and the assumption that [HOx] ~ [HO2},
determine the analytical expressions for [OH], [HO2], and P(O3)
in terms of P(HOx), [NO],
[CO], [O3], and rate coefficients for the three NO regimes. For this problem, P(O3) = kNO+HO2
[NO] [HO2].